Connect both computers over ethernet and rsync the data across. It will still take several hours over gigabit ethernet though.

Quickest -

1. Take the lid off the source PC put the HDD in it
2. Copy the stuff.
3. Pull it out
4. Put it the other PC,
5. Your done

Formatting the HDD my be optional.

1. Take the drive from PC 1 and attach to PC 2 => copy / paste

2. External drive

Parallel port would be faster than serial, but if you’re using serial I’d go with Z modem for the compression and error correction.

What is the best method?

Sometimes the best method isn’t a transfer at all. Don’t forget transporting is an option.
Do you need to transfer the files? or could you just use an external you share between different PCs?
If an external works, but seems inconvenient, you can fix that by having the drive connected to a USB switch. When connected to a switch you can press a button or use a remote to change which PC the drive is connected to giving you instant access to the drive contents without having to sync/copy anything over.

Links below for examples of USB switches
https://www.amazon.com/Cable-Matters-Sharing-Computers-Peripherals/dp/B083JKDNRJ/
https://www.amazon.com/Sabrent-Computers-Peripherals-Indicators-USB-SW30/dp/B074TYDJK2/

If you want the bare minimum fast transfer and both PC are in local network, use Dukto-R6. It’s super basic file copying, you just need to drag and drop.

For more advanced options,the others have already pointed it out.

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I’ve been sending 10TB from one PC to another on my network over the last 2 days, it’s nearly done. It’s a wired network, and while sometimes I use tools like robocopy for more granular control over the the copy settings and logging of any copy errors, I generally find the standard windows copy tool to be faster.

You could go over a wired network.

Fastest “normal” way would be write it to a USB 3 drive on machine 1, read from drive later on machine 2. An SSD would be best. Even with having to do the write and read in two phases, I’d still expect it to be faster than a 1G network.

(Less normal ways would be things like Thundrerbolt SSDs, 10G or 40G ethernet for direct transfer, etc. But if you have that kind of tech already in place, then you’re not asking. ;)

robocopy or rsync if you can’t place the drive in the target or an external enclosure.

Over LAN with flavored solution of your choice.
Other than that, I use one of my spare drives and my USB docking station if I need to move it outside of my own house. I never really had a need for dedicated external drives but a docking station is handy for many things, this being one of them.

External usb hdd

rsync over a wired network. That way, I can stop and resume at any time.

10 GbE. 17 minutes.

Of course you need disks that can read/write at that speed (1.25 GB/s). Should not be a problem for NVMe SSDs.